Metal-pigment complex derived from natural dye of anthocyanin: a potential candidate for DSSC photosensitizer

Authors : Agus Abhi Purwoko; Saprizal Hadisaputra; Veni Rori Setiawati
article cite 4 Year 2019
source: IOP Conference Series Materials Science and Engineering
Abstract

This research is aimed to synthesize iron-pigment complex of anthocyanin extracted from the peel of red dragon fruit (Hylocereus polyrhizus). The targeted iron-complex was then evaluated to confirm its potential use as photosensitizer on Dye Sensitize Solar Cell (DSSC). The electronic absorption spectrum of the red dragon fruit extract showed a broad band spanning from 400 nm to 600 nm and a band maximum at 533 nm. This band was then evaluated to find out the energy of electronic transition; an excitation from highest occupied molecular orbital (HOMO; valence band) toward lowest unoccupied molecular orbital (LUMO; conduction band). The calculation resulted in the equivalent energy level of 1.98 eV for HOMO, and 4.48 eV. These values represent the energy gap (Eg) for sensitizer on DSSC. Furthermore, evaluation of electronic transition of iron complex reveals that there is an increase of absorption coverage range, due in particular the blue shift of the conduction band. These characteristics are supporting evidences that the iron-anthocyanin complex is a good candidate for sensitizer of DSSC.


Concepts :
TiO2 Photocatalysis and Solar Cells
Advanced Photocatalysis Techniques
Transition Metal Oxide Nanomaterials
article cite 4 Year 2019 source IOP Conference Series Materials Science and Engineering
SDGs
Affordable and clean energy
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